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- W245713730 abstract "The general theory of dissociative attachment, vibrational excitation by electron impact, and related reaction processes has been developed by Chen /1/, O’Malley /2/, Bardsley /3/ and others within the framework of Feshbach’s projection operator formalism. In this formulation, the nuclear dynamics in the negative ion is governed by an “optical” potential Vopt which may be written as $$ {V_{{opt}}} = {V_1}(R) + Delta left( {R,E - {H_O}} right) - frac{1}{2}iGamma left( {R,E - {H_O}} right) $$(1)where $$ {H_O} = {T_N} + {v_O}(R) $$(2)$$ Gamma left( {R,E} right) = 2pi {left| {{v_E}(R)} right|^2} $$(3)$$ Delta left( {R,E} right) = frac{P}{{2pi }}int {} dE'Gamma left( {R,E'} right)/left( {E - E'} right) $$(4)Here E is the total energy, R the internuclear distance, TN the nuclear kinetic energy operator, Vo(R) the potential energy curve of the target molecule, and V1 (R) the potential energy curve of a suitable diabatic discrete electronic state of the negative ion /1–3/. The discrete state is coupled via vE(R) to the electronic continuum of the target molecule, which results in a decay width Γ and a level-shift Δ as a given in eqs. (1–4)." @default.
- W245713730 created "2016-06-24" @default.
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- W245713730 date "1984-01-01" @default.
- W245713730 modified "2023-09-26" @default.
- W245713730 title "Calculation of Cross Sections for Dissociative Attachment and Vibrational Excitation in HCl Beyond the Local Complex Potential Approximation" @default.
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- W245713730 doi "https://doi.org/10.1007/978-3-642-46502-4_24" @default.
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