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- W2461109461 abstract "It is highly desirable but challenging to develop bifunctional catalysts for efficiently catalyzing both the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) in energy storage and conversion systems. Here a simple yet cost-effective strategy is developed to fabricate nitrogen and phosphorus dual-doped graphene/carbon nanosheets (N,P-GCNS) with N,P-doped carbon sandwiching few-layers-thick graphene. The as-prepared N,P-GCNS shows outstanding catalytic activity toward both ORR and OER with a potential gap of 0.71 V between the OER potential at a current density of 10 mA cm–2 and the ORR potential at a current density of −3 mA cm–2, illustrating that it is the best metal-free bifunctional electrocatalysts reported to date. The superb bifunctional catalytic performance is attributed to the synergistic effects between the doped N and P atoms, the full exposure of the active sites on the surface of the N,P-GCNS nanosheets, the high conductivity of the incorporated graphene, and the large surf..." @default.
- W2461109461 created "2016-07-22" @default.
- W2461109461 creator A5027105361 @default.
- W2461109461 creator A5042275051 @default.
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- W2461109461 date "2015-06-10" @default.
- W2461109461 modified "2023-10-17" @default.
- W2461109461 title "Nitrogen and Phosphorus Dual-Doped Graphene/Carbon Nanosheets as Bifunctional Electrocatalysts for Oxygen Reduction and Evolution" @default.
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- W2461109461 doi "https://doi.org/10.1021/acscatal.5b00601" @default.
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