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• W2462251503 abstract "Electrocatalytic hydrogenation (ECH) is a sustainable pathway for the synthesis of value-added organic compounds, provided affordable catalysts with high activity, selectivity and durability are developed. Here, we synthesize Cu/C, Ni/C, and CuNi/C nanoparticles and compare their performance to Pt/C, Ru/C, PtRu/C for the ECH of hydroxyacetone, a bio-derived feedstock surrogate containing a carbonyl and a hydroxyl functional group. The non-precious metal electrocatalysts show promising conversion-time behavior, product selectivities, and Faradaic efficiencies. Ni/C forms propylene glycol with a selectivity of 89 % (at 80 % conversion), while Cu/C catalyzes ECH (52 % selectivity) and hydrodeoxygenation (HDO, 48 % selectivity, accounting for evaporation). CuNi/C shows increased turnover frequencies but reduced ECH selectivity (80 % at 80 % conversion) as compared to the Ni/C catalyst. Importantly, stability studies show that the non-precious metal catalysts do not leach at operating conditions." @default.
• W2462251503 created "2016-07-22" @default.
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• W2462251503 date "2016-06-23" @default.
• W2462251503 modified "2023-10-09" @default.
• W2462251503 title "Electrocatalytic Hydrogenation of Oxygenates using Earth‐Abundant Transition‐Metal Nanoparticles under Mild Conditions" @default.
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• W2462251503 doi "https://doi.org/10.1002/cssc.201600290" @default.
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