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- W2466143352 startingPage "2908" @default.
- W2466143352 abstract "An efficient organocascade quadruple reaction was conducted to synthesize a functionalized spiropolycyclic scaffold in high chemical yields (43-80%) and excellent levels of stereoselectivity (up to >19:1 dr and 99% ee). The quadruple reaction proceeded smoothly between 1,3-indanedione and aromatic aldehydes with concomitant desymmetrization of prochiral 4-substituted cyclohexanones through the Knoevenagel/Michael/aldol/aldol reaction sequence catalyzed by a bifunctional thiourea catalyst. Two of the formed products were transformed into spirocyclic epoxides containing four contiguous quaternary centers." @default.
- W2466143352 created "2016-07-22" @default.
- W2466143352 creator A5036599524 @default.
- W2466143352 creator A5048144975 @default.
- W2466143352 creator A5066026484 @default.
- W2466143352 date "2015-05-28" @default.
- W2466143352 modified "2023-09-30" @default.
- W2466143352 title "Enantioselective Synthesis of Functionalized Polycarbocycles via a Three-Component Organocascade Quadruple Reaction" @default.
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- W2466143352 doi "https://doi.org/10.1021/acs.orglett.5b01040" @default.
- W2466143352 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26020799" @default.
- W2466143352 hasPublicationYear "2015" @default.
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