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- W2467023897 abstract "The nucleation of many natural, biogenic, and synthetic crystals involves the initial formation of metastable precursors that provides a kinetic pathway for an amorphous-to-crystalline transformation. This nonclassical mechanism is believed to be the dominant crystallization pathway for microporous zeolites. Despite significant research on zeolite growth mechanisms, molecular level details regarding the assembly, physicochemical properties, and structural evolution of amorphous (alumino)silicate precursors remain elusive. Here we use a combination of diffraction, scattering, and microscopy techniques to characterize the amorphous precursors that assemble and evolve during the synthesis of zeolites FAU and LTA – two materials that are widely used in commercial applications such as catalysis, adsorption, separations, and ion-exchange. Nucleation occurs by a two-step mechanism involving the initial formation of aggregates that serve as heterogeneous sites for nucleation. Using colloidal silica as a reagent, ..." @default.
- W2467023897 created "2016-07-22" @default.
- W2467023897 creator A5051053578 @default.
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- W2467023897 creator A5067095101 @default.
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- W2467023897 date "2016-07-05" @default.
- W2467023897 modified "2023-10-15" @default.
- W2467023897 title "Nucleation of FAU and LTA Zeolites from Heterogeneous Aluminosilicate Precursors" @default.
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- W2467023897 doi "https://doi.org/10.1021/acs.chemmater.6b01000" @default.
- W2467023897 hasPublicationYear "2016" @default.
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