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- W2467581379 abstract "Perfectly ordered states are targets in diverse molecular to microscale systems involving, for example, atomic clusters, protein folding, protein crystallization, nanoparticle superlattices, and colloidal crystals. However, there is no obvious approach to control the assembly of perfectly ordered global free energy minimum structures; near-equilibrium assembly is impractically slow, and faster out-of-equilibrium processes generally terminate in defective states. Here, we demonstrate the rapid and robust assembly of perfect crystals by navigating kinetic bottlenecks using closed-loop control of electric field mediated crystallization of colloidal particles. An optimal policy is computed with dynamic programming using a reaction coordinate based dynamic model. By tracking real-time stochastic particle configurations and adjusting applied fields via feedback, the evolution of unassembled particles is guided through polycrystalline states into single domain crystals. This approach to controlling the assembly of a target structure is based on general principles that make it applicable to a broad range of processes from nano- to microscales (where tuning a global thermodynamic variable yields temporal control over thermal sampling of different states via their relative free energies)." @default.
- W2467581379 created "2016-07-22" @default.
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- W2467581379 date "2016-07-11" @default.
- W2467581379 modified "2023-10-11" @default.
- W2467581379 title "Optimal Feedback Controlled Assembly of Perfect Crystals" @default.
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- W2467581379 doi "https://doi.org/10.1021/acsnano.6b02400" @default.
- W2467581379 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27387146" @default.
- W2467581379 hasPublicationYear "2016" @default.
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