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- W2467858105 abstract "Perovskite-shelled colloidal quantum dots (CQDs) with low trap-state density are promising candidates for large-scale, low-cost, and lightweight solar cell applications. However, even minimal trap states can significantly limit CQD-based solar cell efficiency. We reported trap-state-mediated exciton transports in methylammonium lead triiodide (MAPbI3) perovskite-passivated PbS CQD thin films. Excitation power-dependent photocarrier radiometry (PCR) intensity study demonstrated the free (electrons/holes)-to-bound (acceptors/donors) and trap-state-related transition-induced nonlinear response of CQD thin films to excitation. The existence of shallow trap states (activation energy: 33.8–40.7 meV) was characterized using photothermal emission spectra at different modulation frequencies. CQD thin films were imaged, for the first time, by InGaAs-camera-based nondestructive homodyne and heterodyne lock-in carrierographies (LIC; spectrally gated dynamic photoluminescence imaging), clearly showcasing photocarrier ..." @default.
- W2467858105 created "2016-07-22" @default.
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- W2467858105 date "2016-06-27" @default.
- W2467858105 modified "2023-09-24" @default.
- W2467858105 title "Quantitative Analysis of Trap-State-Mediated Exciton Transport in Perovskite-Shelled PbS Quantum Dot Thin Films Using Photocarrier Diffusion-Wave Nondestructive Evaluation and Imaging" @default.
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- W2467858105 doi "https://doi.org/10.1021/acs.jpcc.6b04468" @default.
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