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• W2470683402 abstract "The discovery of a light-induced spin transition at cryogenic temperatures in a series of iron(II) spin-crossover compounds in 1984 has had an enormous impact on spin-crossover research. Apart from being an interesting photophysical phenomenon in its own right, it provided the means of studying the dynamics of the intersystem crossing process between the high-spin and the low-spin state in a series of compounds and over a large temperature range. It could thus be firmly established that intersystem crossing in spin-crossover compounds is a tunnelling process, with a limiting low-temperature lifetime below 50 K and a thermally activated region above 100 K. This review begins with an elucidation of the mechanism of the light-induced spin transition, followed by an in depth discussion of the chemical and physical factors, including cooperative effects, governing the lifetimes of the light-induced metastable states.Open image in new window" @default.
• W2470683402 created "2016-07-22" @default.
• W2470683402 creator A5069029201 @default.
• W2470683402 date "2012-02-24" @default.
• W2470683402 modified "2023-10-13" @default.
• W2470683402 title "Light-Induced Spin Crossover and the High-Spin→Low-Spin Relaxation" @default.
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• W2470683402 doi "https://doi.org/10.1007/b95416" @default.
• W2470683402 hasPublicationYear "2012" @default.
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