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• W2471563531 abstract "Phase-sensitive sum-frequency vibrational spectroscopy was used to probe interfaces of a long-chain alcohol monolayer with various electrolytic solutions, chosen as a prototype for nonionic organic/water interfaces. Spectra in the OH stretching range were observed to be under the influence of ions emerging at the interfaces. Analysis of the spectra with the help of Levin’s theory allowed us to quantitatively find the surface densities of various ions and, hence, the ion affinities and surface pH/pOH at the alcohol/water interface. For the ions studied, the interface affinity has the ranking order of OH– > I– > Cl– ∼ H3O+ > Na+, the same as that at the air/water interface except that OH– and H3O+ have their places interchanged. Significantly stronger affinity of OH– than H3O+ with the result of surface pH/pOH extrapolating to bulk pH 7 suggests that the alcohol/neutral water interface is weakly basic." @default.
• W2471563531 created "2016-07-22" @default.
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• W2471563531 date "2016-07-06" @default.
• W2471563531 modified "2023-10-16" @default.
• W2471563531 title "Surface pH and Ion Affinity at the Alcohol-Monolayer/Water Interface Studied by Sum-Frequency Spectroscopy" @default.
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• W2471563531 doi "https://doi.org/10.1021/acs.jpcc.6b04449" @default.
• W2471563531 hasPublicationYear "2016" @default.
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