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• W2471660587 abstract "Abstract This paper reports the photoelectrocatalytic activities of a ruthenated porphyrin [Ru(phen) 2 (IP-C 4 O-TPP)] 2+ (denoted as Ru(II)PTPP, phen = 1,10-phenanthroline, IP = imidazo[4,5- f ][1,10]phenanthroline and TPP = 5,10,15,20-tetraphenylporphyrin) containing a covalently-linked butoxy chain (-C 4 O-) between IP and TPP moieties by means of various electrochemical techniques in combination with absorption spectroscopy and scanning electronic microscopy. Ru(II)PTPP is assembled on the surface of CdS nanoparticles, showing two Ru(II)-based peaks at 0.296 V and 0.830 V, where uric acid (UA) can be photoelectrocatalytically oxidized in a linear range of 0.01-10.0 mmol L −1 . The −C 4 O- chain endows the Ru(II)PTPP/carbon felt (CF) electrode with favorable dioxygen (O 2 ) binding sites to achieve a couple of new redox peaks at −0.213 V, where O 2 involves electrocatalytic reduction reactions. While employing 5.0 mmol L −1 UA as fuel, and 60 mL min −1 O 2 as oxidant, the proposed photoelectrochemical fuel cell shows open-circuit photovoltage of 0.656 V, short-circuit photocurrent density of 0.136 mA cm −2 , and maximum power density of 31.50 μW cm −2 at 0.497 V under visible-light illumination of 0.18 mW cm −2 . The present study provides an interesting platform for the utilization of renewable energy sources." @default.
• W2471660587 created "2016-07-22" @default.
• W2471660587 creator A5010214831 @default.
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• W2471660587 date "2016-09-01" @default.
• W2471660587 modified "2023-09-23" @default.
• W2471660587 title "Unique catalytic properties of a butoxy chain-containing ruthenated porphyrin towards oxidation of uric acid and reduction of dioxygen for visible light-enhanced fuel cells" @default.
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• W2471660587 doi "https://doi.org/10.1016/j.electacta.2016.06.147" @default.
• W2471660587 hasPublicationYear "2016" @default.
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