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- W2473119684 abstract "Discovery of novel compounds capable of electrochemical ion intercalation is a primary step toward development of advanced electrochemical devices such as batteries. Although cyano-bridged coordination polymers including Prussian blue analogues have been intensively investigated as ion intercalation materials, the solid-state electrochemistry of the octacyanotungstate-bridged coordination polymer has not been investigated. Here, we demonstrate that an octacyanotungstate-bridged coordination polymer Tb(H2O)5[W(CN)8] operates as a Li+-ion intercalation electrode material. The detailed magnetic measurements reveal that the tunable amount of intercalated Li+ ion in the solid-state redox reaction between paramagnetic [WV(CN)8]3– and diamagnetic [WIV(CN)8]4– in the framework enables the electrochemical control of different magnetic regimes. While the initial ferromagnetic long-range ordering is irreversibly lost upon lithium insertion, electrochemical switching between paramagnetic and short-range ordering regimes can be achieved." @default.
- W2473119684 created "2016-07-22" @default.
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- W2473119684 date "2016-07-15" @default.
- W2473119684 modified "2023-10-13" @default.
- W2473119684 title "Electrochemical Li-Ion Intercalation in Octacyanotungstate-Bridged Coordination Polymer with Evidence of Three Magnetic Regimes" @default.
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- W2473119684 doi "https://doi.org/10.1021/acs.inorgchem.6b01086" @default.
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