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• W2473131502 endingPage "2505" @default.
• W2473131502 startingPage "2482" @default.
• W2473131502 abstract "The large alkaline earths (Ae), calcium, strontium and barium, have in the past 15 years yielded a brand new generation of heteroleptic molecular catalysts for the production of fine chemicals. However, the integrity of these complexes is often plagued by ligand redistribution equilibria in solution. This personal account retraces the paths followed in our research group towards the design of stable heteroleptic alkalino-earth complexes, including the use of intramolecular noncovalent Ae···H-Si and Ae···F-C interactions. Their implementation as homogenous precatalysts for reactions such as the intramolecular and intermolecular hydroamination and hydrophosphination of activated alkenes, the hydrophosphonylation of ketones, and the dehydrogenative coupling of amines and hydrosilanes that enable the efficient and controlled formations of CP, CN, or SiN σ-bonds, is presented in a synthetic perspective that highlights their overall outstanding catalytic performance." @default.
• W2473131502 created "2016-07-22" @default.
• W2473131502 creator A5057429214 @default.
• W2473131502 creator A5064611725 @default.
• W2473131502 date "2016-06-29" @default.
• W2473131502 modified "2023-10-18" @default.
• W2473131502 title "Calcium, Strontium and Barium Homogeneous Catalysts for Fine Chemicals Synthesis" @default.
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