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• W2473919837 abstract "The application of MnOx-CeO2 as the low temperature selective catalytic reduction (SCR) catalyst to control NOx emission from coal-fired power plants is extremely restricted due to the unrecoverable deactivation by SO2. There is little SO2 in the flue gas from biomass-fired power plants, and the concentration of alkali metals in the flue gas after the electrostatic precipitator is very low, so the application of MnOx-CeO2 may be possible to control NOx emission from biomass-fired power plants. However, a very small amount of alkali metals showed a seriously negative effect on NO reduction over MnOx-CeO2 such that both NOx conversion and N2 selectivity obviously decreased. In this work, the mechanism of NO reduction over MnOx-CeO2 and K-MnOx-CeO2 was investigated by the transient reaction study and the kinetic parameters of NO reduction were obtained from the steady-state kinetic study. After comparison of the kinetic parameters, the mechanism of potassium deactivation on NO reduction over MnOx-CeO2 was discovered. The decrease of the SCR activity of MnOx-CeO2 after potassium deactivation was mainly attributed to the decrease of acid site and Mn4+ concentration on the surface, and the increase of N2O selectivity was mainly related to the occurrence of N2O formation over K-MnOx-CeO2 through the Langmuir–Hinshelwood mechanism." @default.
• W2473919837 created "2016-07-22" @default.
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• W2473919837 date "2016-07-12" @default.
• W2473919837 modified "2023-09-26" @default.
• W2473919837 title "Alkali Metal Deactivation on the Low Temperature Selective Catalytic Reduction of NO_<i>x</i> with NH₃ over MnO_<i>x</i>-CeO₂: A Mechanism Study" @default.
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• W2473919837 doi "https://doi.org/10.1021/acs.jpcc.6b05175" @default.
• W2473919837 hasPublicationYear "2016" @default.
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