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• W2475994872 abstract "Recent advances for the construction of heterocyclic scaffolds via the transition metal-catalyzed carbonylative CH functionalization have been summarized and discussed. Based on the transition metal catalysts applied such as cobalt, ruthenium, rhodium, and palladium, we then subclassify the chapter according to the size of the ring formed, thus four-, five-, and six-membered ring heterocycles. Solutions to the palladium-catalyzed carbonylation challenges include the (i) utilization of unique ligand such as special α-amino acid, (ii) employment of cationic Pd(II) precursor which could enhance the nucleophilic attack of the CH bond toward the palladium center, and (iii) usage of acid as solvent or additive which also favors the generation of cationic palladium center. All the reaction conditions as well as the scope and limitation of every procedure have been listed. Representative reaction mechanisms have been discussed as well." @default.
• W2475994872 created "2016-08-23" @default.
• W2475994872 creator A5014543294 @default.
• W2475994872 creator A5075108316 @default.
• W2475994872 date "2016-01-27" @default.
• W2475994872 modified "2023-10-18" @default.
• W2475994872 title "Transition Metal-Catalyzed Carbonylative Synthesis of Heterocycles via CH Activation" @default.
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• W2475994872 doi "https://doi.org/10.1002/9783527691920.ch15" @default.
• W2475994872 hasPublicationYear "2016" @default.
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