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- W2476497817 abstract "Direct observations of heterogeneous catalytic processes on a molecular level only became possible with the advent of new spectroscopic techniques and in particular, by utilizing several techniques in concert on a given catalytic process. Combining such spectroscopic investigations with concomitant kinetic investigations provides new insights into the solid state and surface mechanisms of selective olefin oxidation catalysis by mixed metal oxides. The application of multiple techniques including Raman, infrared, XRD, neutron diffraction, and XPS has provided direct evidence of several key aspects of the propylene to acrylonitrile ammoxidation mechanism over bismuth molybdate based catalysts. The mechanistic insights include: 1) direct spectroscopic evidence for solid state disproportionation of the metastable Bi2Mo2O9 phase under redox conditions, 2) identification of key catalytic phases in bismuth-iron molybdate systems, and 3) direct identification of catalytic function of active oxide ions in bismuth molybdate selective olefin oxidation catalysts." @default.
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- W2476497817 date "1985-10-16" @default.
- W2476497817 modified "2023-10-11" @default.
- W2476497817 title "Correlation Between Spectroscopic Measurements and Catalytic Behavior of Selective Oxidation Catalysts" @default.
- W2476497817 doi "https://doi.org/10.1021/bk-1985-0288.ch003" @default.
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