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• W2477980016 abstract "Zn- and Na-modulated Fe catalysts were fabricated by a simple coprecipitation/washing method. Zn greatly changed the size of iron species, serving as the structural promoter, while the existence of Na on the surface of the Fe catalyst alters the electronic structure, making the catalyst very active for CO activation. Most importantly, the electronic structure of the catalyst surface suppresses the hydrogenation of double bonds and promotes desorption of products, which renders the catalyst unexpectedly reactive toward alkenes-especially C5+ alkenes (with more than 50% selectivity in hydrocarbons)-while lowering the selectivity for undesired products. This study enriches C1 chemistry and the design of highly selective new catalysts for high-value chemicals." @default.
• W2477980016 created "2016-08-23" @default.
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• W2477980016 date "2016-07-22" @default.
• W2477980016 modified "2023-10-15" @default.
• W2477980016 title "Highly Tunable Selectivity for Syngas-Derived Alkenes over Zinc and Sodium-Modulated Fe₅C₂Catalyst" @default.
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• W2477980016 doi "https://doi.org/10.1002/anie.201603556" @default.
• W2477980016 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27445106" @default.
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