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• W2480561679 startingPage "21366" @default.
• W2480561679 abstract "Dopamine, which can be electrochemically oxidized to polydopamine on cathode surface, was introduced as an electrolyte additive for high-voltage lithium-ion batteries (LIBs). The addition of 0.1 wt % dopamine to the electrolyte led to the formation of a polydopamine-containing layer on the cathode, thereby resulting in suppression of the oxidative decomposition of the electrolyte during high-voltage operation (up to 4.5 V) of a LiNi1/3Co1/3Mn1/3O2/artificial graphite cell. The addition of dopamine to the electrolyte improved the capacity retention of the cell from 136 to 147 mAh g–1 after 100 cycles at a rate of 1 C and a cutoff voltage of 4.5 V, while the cycle performance and rate capability with a cutoff voltage of 4.3 V were comparable to those of the cell without dopamine. Further evidence of the positive impact of dopamine on high-voltage LIBs was the lower DC-IRs and AC impedances, as well as the retention of the cathode morphology even after operation at 4.5 V." @default.
• W2480561679 created "2016-08-23" @default.
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• W2480561679 date "2016-08-10" @default.
• W2480561679 modified "2023-10-13" @default.
• W2480561679 title "Dopamine as a Novel Electrolyte Additive for High-Voltage Lithium-Ion Batteries" @default.
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• W2480561679 doi "https://doi.org/10.1021/acsami.6b06074" @default.
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