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- W2486984920 abstract "Transient fluorescence spectroscopy on nanosecond and picosecond time scales has been used in an attempt to study the pathways of excitation energy transport (EET) and trapping for poly-(1-vinylnaphthalene), p-VN, and poly-(N-vinylc arbazole), p-N-VCz, in dilute fluid solution. Excited state localization has been probed by collecting the transient fluorescence patterns of excimer-forming-sites (EFS) in typical trapping experiments. Fluorescence rise-profiles of both mobile and static excimers have been analyzed on the premises of low-dimensional transport topology and effective diagonal disorder of aromatic hopping sites. A trapping function of the form k(t) = b + ct-1/2, a distribution of transport states {X1} and a small ensemble of energy-relaxed, monomeric tail-states have been processed in kinetic schemes. The calculated profiles are nonexponential and can recover satisfactorily the experimental curves. The rationale behind - a time-dependent excited-state random walk among energy-dispersive chromophores - has been discussed. Electronic excitations in molecular aggregates have received considerable attention from" @default.
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- W2486984920 date "1987-07-23" @default.
- W2486984920 modified "2023-10-13" @default.
- W2486984920 title "Electronic Energy Relaxation in Aromatic Vinyl Homopolymers" @default.
- W2486984920 doi "https://doi.org/10.1021/bk-1987-0358.ch018" @default.
- W2486984920 hasPublicationYear "1987" @default.
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