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- W2488337983 abstract "on the basis of population rate equation of multiphoton ionization and fragmentation processes, the controllability of fragmentation process in mpi experiments of polyatomic molecules is analyzed in this paper. curves of ionization efficiency and mean energy of ions versus laser intensity were calculated for different ionization schemes. from the calculation results, we find that only 1+1 ionization scheme, soft ionization and hard fragmentation can be controlled by changing the intensity of ionization laser. for 3+1 ionization scheme, due to additional absorption photons after ionization, the ions have already obtained internal energy about 20 similar to 30ev/per ion even at single ion detection limit. this amount of energy far exceeds the dissociation threshold of the parent ion, so the parent ions formed by ionization can completely dissociate to daughters in the same laser pules. our analyses can explain why parent ions didn't appear in mpi mass spectra of furan molecule at 450 nm." @default.
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- W2488337983 date "1995-01-01" @default.
- W2488337983 modified "2023-09-26" @default.
- W2488337983 title "Population Rate Equation Analysis of Controllability of Fragmentation Process in Multiphoton Ionization Experiments of Polyatomic Molecules" @default.
- W2488337983 doi "https://doi.org/10.3866/pku.whxb19950203" @default.
- W2488337983 hasPublicationYear "1995" @default.
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