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- W2488550089 abstract "By providing an in-situ measure of the concentrations and lifetimes of surface intermediates, transient isotope tracing provides a strong link between surface science, other spectroscopic investigations and catalytic reaction mechanisms. A brief discussion of the method is followed by recent results on methane oxidation catalysis to demonstrate its use. Mixed metal (Bi/Sn,Pb/Ta) oxide catalysts with the pyrochlore structure as well as lithium-magnesia were studied. The catalysts show an immeasurably small (<0.01) surface coverages by carbon-containing intermediates. These catalysts, like others, rapidly exchange their surface oxygen with the bulk, as well with the gas phase, particularly with CO2. These exchange reactions obscure much of the variation in surface oxygen species reactivity." @default.
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- W2488550089 date "1992-01-23" @default.
- W2488550089 modified "2023-09-25" @default.
- W2488550089 title "In Situ Surface Kinetics by Dynamic Isotopic Tracing" @default.
- W2488550089 doi "https://doi.org/10.1021/bk-1992-0482.ch015" @default.
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