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- W2488579810 abstract "While glassy dynamics and (ionic) charge transport coincide in low-molecular weight ionic liquids (ILs), they are widely decoupled in corresponding polymeric systems. This is studied by means of broadband dielectric spectroscopy (BDS) for monovalent and bivalent telechelic polyisobutylene (PIB) carrying the Ionic Liquid (IL)-like cationic headgroup (N,N,N-triethylammonium or 1-methylpyrrolidinium) with Br, NTf2, OTf or pTOS as anions, as well as for neat and polymerized 1-vinyl-3-pentylimidazolium bis-(trifluoromethylsulfonyl) imide (PVIM NTf2). The former shows a wealth of dielectrically active fluctuations in contrast to the latter, where only the dynamic glass transition is observed. Additionally a conductivity relaxation originating from charge transport in the IL-like moieties and a weak electrode polarization caused by the accumulation of mobile charge carriers at the metal interfaces is found. In both systems molecular fluctuations and charge transport are well separated from each other thereby enabling accurate description of the net conductivity within the framework of the effective medium approximation for the PIB-based systems." @default.
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- W2488579810 date "2016-01-01" @default.
- W2488579810 modified "2023-09-25" @default.
- W2488579810 title "Glassy Dynamics and Charge Transport in Polymeric Ionic Liquids" @default.
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- W2488579810 doi "https://doi.org/10.1007/978-3-319-32489-0_5" @default.
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