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- W2489389689 abstract "This work demonstrates that threshold voltage (VT) of organic thin-film transistors (OTFTs) can be controlled systematically by introducing new copolymer dielectrics with electropositive functionality. A series of homogeneous copolymer dielectrics are polymerized from two monomers, 1,3,5-trimethyl-1,3,5-trivinyl cyclotrisiloxane (V3D3) and 1-vinylimidazole (VI), via initiated chemical vapor deposition. The chemical composition of the copolymer dielectrics is exquisitely controlled to tune the VT of C60 OTFTs. In particular, all the copolymer dielectrics demonstrated in this work exhibit extremely low leakage current densities (lower than 2.5 × 10−8 A cm−2 at ±3 MV cm−1) even with a thickness less than 23 nm. Furthermore, by introducing an ultrathin pV3D3 interfacial layer (about 3 nm) between the copolymer dielectrics and C60 semiconductor, the high mobility of the C60 OTFTs (about 1 cm2 V−1 s−1) remains unperturbed, showing that VT can be controlled independently by tuning the composition of the copolymer dielectrics. Coupled with the ultralow dielectric thickness, the independent VT controllability allows the VT to be aligned near 0 V with sub-3 V operating voltage, which enables a substantial decrease of device power consumption. The suggested method can be employed widely to enhance device performance and reduce power consumption in various organic integrated circuit applications." @default.
- W2489389689 created "2016-08-23" @default.
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- W2489389689 date "2016-08-03" @default.
- W2489389689 modified "2023-09-26" @default.
- W2489389689 title "Synthesis of Ultrathin, Homogeneous Copolymer Dielectrics to Control the Threshold Voltage of Organic Thin-Film Transistors" @default.
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- W2489389689 doi "https://doi.org/10.1002/adfm.201602585" @default.
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