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• W2490521515 startingPage "7320" @default.
• W2490521515 abstract "A ruthenium(II) flavonolate complex, [RuII(bpy)2fla][BF4], was synthesized to model the reactivity of the flavonol dioxygenases. The treatment of dry CH3CN solutions of [RuII(bpy)2fla][BF4] with dioxygen under light leads to the oxidative O-heterocyclic ring opening of the coordinated substrate flavonolate, resulting in the formation of [RuII(bpy)2(carboxylate)][BF4] (carboxylate = O-benzoylsalicylate or benzoate) species, as determined by electrospray ionization mass spectrometry. Moderation of the excitation and temperature allowed isolation and characterization of an intermediate, [RuII(bpy)2bpg][BF4] (bpg = 2-benzoyloxyphenylglyoxylate), generated by the 1,2-addition of dioxygen to the central flavonolate ring." @default.
• W2490521515 created "2016-08-23" @default.
• W2490521515 creator A5047205376 @default.
• W2490521515 creator A5049835071 @default.
• W2490521515 creator A5077214849 @default.
• W2490521515 date "2016-07-20" @default.
• W2490521515 modified "2023-09-26" @default.
• W2490521515 title "Characterization of the Initial Intermediate Formed during Photoinduced Oxygenation of the Ruthenium(II) Bis(bipyridyl)flavonolate Complex" @default.
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• W2490521515 doi "https://doi.org/10.1021/acs.inorgchem.6b00852" @default.
• W2490521515 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27437831" @default.
• W2490521515 hasPublicationYear "2016" @default.
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