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- W2500131490 abstract "Metallic nickel nanoparticles well dispersed in graphitized carbon matrix ([email protected]) by pyrolysis of metal-organic frameworks and leaching treatment of hydrochloric acid could greatly enhance the photocatalytic activity of g-C3N4 under visible light irradiation. For 2.0 wt% [email protected]/g-C3N4, the average hydrogen evolution rate is 2.15 mmol h−1 g−1, which is around 88 times higher than that of pure g-C3N4, and even better than that of platinum-loaded g-C3N4. The remarkably improved photocatalytic activities through loading [email protected] can be attributed to the cooperative work of Ni nanoparticles and graphene layers, which facilitate the separation of photo-generated carriers and suppress the recombination of the electron-hole pairs. In addition, the hollow onion-like structure can restrain the formation of Ni-hydrogen bonds which modulates desorption of hydrogen. Our studies may open up a promising strategy to design economical noble-metal-free co-catalysts for efficient solar energy conversion." @default.
- W2500131490 created "2016-08-23" @default.
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- W2500131490 date "2017-01-01" @default.
- W2500131490 modified "2023-10-16" @default.
- W2500131490 title "Nickel nanoparticles coated with graphene layers as efficient co-catalyst for photocatalytic hydrogen evolution" @default.
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- W2500131490 doi "https://doi.org/10.1016/j.apcatb.2016.07.033" @default.
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