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• W2500970825 abstract "Rainbow structures in the scattering angular distribution play an important role in deepening our understanding about the elastic and rotationally inelastic collisions of atoms/molecules. Reported here is the discovery of a rainbow in a chemical reaction. At Ec = 4.3 kcal mol–1 one of the correlated product pairs in the F + CH3D reaction, (vHF, vCH2D) = (3, 00), displays a distinct bulge in angular distribution. We showed that the bulge originates predominantly from the low-j states of the HF(v = 3) products. Heuristic considerations led us to propose that such a bulge could be regarded as a signature for rainbow scattering. The underlying mechanism for its occurrence in this nearly thermoneutral product pair is ascribed to a delicate interplay of the attractive and repulsive parts of interactions in the vicinity of the transition state. In a sense, the situation bears striking similarity to the more familiar elastic rainbow, thus coined “reactive rainbow”." @default.
• W2500970825 created "2016-08-23" @default.
• W2500970825 creator A5043161715 @default.
• W2500970825 creator A5068698532 @default.
• W2500970825 date "2016-08-19" @default.
• W2500970825 modified "2023-10-18" @default.
• W2500970825 title "Observation of a Reactive Rainbow in F + CH₃D → CH₂D(<i>v</i> = 0) + HF(<i>v</i> = 3)?" @default.
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• W2500970825 doi "https://doi.org/10.1021/acs.jpca.6b07772" @default.
• W2500970825 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27509923" @default.
• W2500970825 hasPublicationYear "2016" @default.
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