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- W2506331211 abstract "Molecular beam techniques have been employed to study the dissociative chemisorption dynamics of a number of systems with particular regard to understanding the effect of surface temperature on the probability of this process. It is now apparent that this parameter can affect the outcome of potentially reactive gas-surface encounters in a number of different ways. These include effects on the trapping probability into weakly bound states, the fraction of adsorbed molecules that proceed to dissociate, and even the probability of direct dissociative chemisorption. We illustrate these findings with reference to studies of the dissociation of N2 on W(100) (which proceeds via a precursor at low kinetic energies), of N2 on Fe(111) and O2 on Pt(111) (both of which involve dissociation via an intermediate state that is accessed only at high kinetic energies), and of CH4 on Pt(111) (where we believe that direct dissociation occurs)." @default.
- W2506331211 created "2016-08-23" @default.
- W2506331211 creator A5049857121 @default.
- W2506331211 date "1992-01-23" @default.
- W2506331211 modified "2023-09-25" @default.
- W2506331211 title "Molecular-Beam Studies of the Effect of Surface Temperature on the Probability of Dissociative Chemisorption" @default.
- W2506331211 doi "https://doi.org/10.1021/bk-1992-0482.ch002" @default.
- W2506331211 hasPublicationYear "1992" @default.
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