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- W2507235514 abstract "This work studied the performance of Ni catalysts supported on three different zirconia structures for SR of toluene, methane and methane/toluene mixtures. The presence of both reactants in the feed decreased the conversion of toluene and methane. This was due to the increase in the concentration of CHx species on the surface of the metallic particle. All Ni/ZrO2 catalysts deactivated during SR of toluene, methane or the mixture. Scanning electron microscopy and thermogravimetric analysis revealed the formation of carbon deposits over the surface of catalysts. However, the amount of carbon deposited depended on the reaction conditions and the structure of zirconia. Monoclinic zirconia exhibits a lower densitiy of acid sites and a higher degree of hydration, which contributes to the lower carbon formation. The amount of carbon deposited over all catalysts significantly increased during SR of the mixture. This is due to a decrease in the rate of the gasification reaction and an increase in the rate of the CHx species formation reaction, which enhances the catalysts deactivation rate." @default.
- W2507235514 created "2016-09-16" @default.
- W2507235514 creator A5014897862 @default.
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- W2507235514 date "2017-07-01" @default.
- W2507235514 modified "2023-10-07" @default.
- W2507235514 title "Steam reforming of toluene, methane and mixtures over Ni/ZrO 2 catalysts" @default.
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- W2507235514 doi "https://doi.org/10.1016/j.cattod.2016.08.024" @default.
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