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• W2509171852 abstract "The application of high-voltage cathode materials in lithium-ion batteries is of high interest to increase the batteries energy density. The cathode material LiNi0.5Mn1.5O4 is a promising candidate, but very different electrochemical results are reported in literature. After all, this differences are highly depending on the specific synthesis route. But, for a final commercialization, a fundamental understanding is lacking, which is needed to optimize the particle morphology for slurry and electrode fabrication on one hand, and regarding the electrochemical properties on the other. In this study, the synthesis of the high-voltage cathode material LiNi0.5Mn1.5O4 by spray drying and its successful application in lithium-ion batteries are presented. The focus is on discussing the influence of two different synthesis routes, namely the application of different precursor compositions, on particle morphology and finally on electrochemical properties. It is shown that by using mixed precursors of acetates and nitrates a higher specific capacity is achieved compared to a route using only acetates. The deviating electrochemical behavior is connected with the different Mn3+ content observed in the samples. The relationship between electrochemical properties and particle morphology is consequently discussed." @default.
• W2509171852 created "2016-09-16" @default.
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• W2509171852 date "2016-05-31" @default.
• W2509171852 modified "2023-09-26" @default.
• W2509171852 title "The Influence of the Synthesis Route on Electrochemical Properties of Spinel Type High-Voltage Cathode Material LiNi_0.5Mn_1.5O₄for Lithium Ion Batteries" @default.
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• W2509171852 doi "https://doi.org/10.1002/9781119234531.ch18" @default.
• W2509171852 hasPublicationYear "2016" @default.
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