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- W2510172168 abstract "Absorption saturation due to surface plasmon resonance affects the optical limiting efficiency of metal nanoparticles (NPs) by raising the limiting threshold to higher laser fluences. It has been shown that in gold, compared to the larger NPs, smaller quantum clusters (QCs) exhibit better optical limiting with lower limiting thresholds due to the absence of absorption saturation. Here we report optical limiting properties of two novel materials, namely, nine-atom silver (Ag9) QCs and graphitic carbon nitride (GCN) nanosheets. The relatively large nonlinear absorption of Ag9 QCs compared to Ag NPs is revealed from open-aperture Z-scan measurements carried out using 532 nm, 5 ns laser pulses. Optical nonlinearity in the QCs arises mostly from free carrier absorption and a relatively weak saturable absorption. The superior limiting efficiency of Ag9 QCs is complemented by excellent chemical stability, which makes silver quantum clusters ideal candidates for optical limiting applications. The two-dimensional ..." @default.
- W2510172168 created "2016-09-16" @default.
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- W2510172168 date "2015-07-02" @default.
- W2510172168 modified "2023-09-27" @default.
- W2510172168 title "Nonlinear Optical Investigations in Nine-Atom Silver Quantum Clusters and Graphitic Carbon Nitride Nanosheets" @default.
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- W2510172168 doi "https://doi.org/10.1021/acs.jpcc.5b02372" @default.
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