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- W2510183342 abstract "The adsorption of C60-malonic derivatives C61(CO2H)2 and C66(CO2H)12 on Au(111) and a pentafluorobenzenethiol-modified Au substrate (PFBT@Au) has been investigated using scanning tunneling microscopy (STM) at a liquid-solid interface. Monofunctionalized C61(CO2H)2 forms a hexagonal close-packed overlayer on Au(111) and individual aligned dimers on PFBT@Au(111). The difference is attributed to the nature of the substrateC61(CO2H)2 interaction (isotropic π-Au bonding vs. anisotropic PFBTCOOH interactions). Surprisingly, in both cases, the directionality of the COOHCOOH motif is compromised in favor of synergistic van der Waals/H bonding interactions. Such van der Waals contacts are geometrically unfeasible in hexafunctionalized C66(CO2H)12 and its assembly on Au(111) leads to a 2D molecular network controlled exclusively by H bonding. For both molecules, the free CO2H groups on the monolayer surface can engage in out-of-plane H bonding interaction resulting in the epitaxial growth of subsequent molecular layers." @default.
- W2510183342 created "2016-09-16" @default.
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- W2510183342 date "2016-01-01" @default.
- W2510183342 modified "2023-09-24" @default.
- W2510183342 title "Hydrogen bonding vs. molecule–surface interactions in 2D self-assembly of [C60]fullerenecarboxylic acids" @default.
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- W2510183342 doi "https://doi.org/10.1039/c6nr04115a" @default.
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