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• W2510457822 abstract "We present a systematic study of morphological changes in monolayers of a rod-like polypeptide (poly-γ-benzyl-L-glutamate (PBLG)) on a Langmuir trough as a function of increasing surface density. Through the combination of atomic force and Brewster angle microscopy, we accessed structural information on the nano- and micro-scale. Already during the spreading process, aggregates formed, leading to a coexistence of randomly organized domains, consisting of preferentially oriented fibers, embedded in a less ordered matrix of lower density. The resulting morphology after spreading resembles a structure of a 2D foam as observed for small amphiphilic molecules. With increasing surface density, we observed that the domains became larger with fibers showing a strong tendency to coarsen. Due to this coarsening process, the plateau region of the surface pressure isotherm exhibited a continuous increase in width of the fibers. In the region of highest surface density, solid-like films composed of compacted wide fibers were observed. These fibers, which were most likely in a glassy state, were fully oriented orthogonal to the compression direction." @default.
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• W2510457822 date "2016-12-01" @default.
• W2510457822 modified "2023-09-25" @default.
• W2510457822 title "Self-assembly behavior of a rod-like polypeptide at the air-water interface" @default.
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• W2510457822 doi "https://doi.org/10.1016/j.polymer.2016.08.023" @default.
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