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- W2511604889 abstract "We present a complete theoretical framework for the axial dispersion of a Brownian colloidal suspension confined in a parallel plate channel, extending the Taylor-Aris treatment to particles with diameters comparable to the channel width. The theoretical model incorporates the effects of confinement on the colloid distribution, corrections to the velocity profile due to the effects of colloid concentration on the suspension viscosity, and position-dependent diffusivities. We test the theoretical model using explicit-solvent molecular dynamics simulations that fully incorporate hydrodynamic correlations and thermal fluctuations and obtain good quantitative agreement between theory and simulations. We find that the nonuniform colloid distributions that arise in confinement due to excluded volume between the colloids and channel walls significantly impact the axial dispersion.3 MoreReceived 29 April 2016DOI:https://doi.org/10.1103/PhysRevFluids.1.044203©2016 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasDiffusionMicrofluidicsPhysical SystemsColloidsTechniquesMolecular dynamicsFluid DynamicsPolymers & Soft Matter" @default.
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- W2511604889 date "2016-08-19" @default.
- W2511604889 modified "2023-10-18" @default.
- W2511604889 title "Axial dispersion of Brownian colloids in microfluidic channels" @default.
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- W2511604889 doi "https://doi.org/10.1103/physrevfluids.1.044203" @default.
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