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• W2511701116 abstract "Nitrogen-doped carbon nanoparticles (NCNPs) were synthesized by a solution plasma process followed by a thermal annealing at 900 °C. Cyano-aromatic molecules, including cyanobenzene (C7H5N), 2-cyanopyridine (C6H4N2), and cyanopyrazine (C5H3N3), were used as single source precursors for the synthesis. The morphological features of NCNPs were governed by the aggregates and agglomerates of uniform nanosized particles (20−40 nm). The structural analyses confirmed that NCNPs mainly exhibited a disordered amorphous carbon structure. The nitrogen doping contents determined from an X-ray photoelectron spectroscopy were found to be 0.58, 1.36, and 1.29 at% for NCNPs synthesized from cyanobenzene, 2-cyanopyridine, and cyanopyrazine, respectively. The improvements of oxygen reduction reaction activity and selectivity toward a four-electron pathway in an alkaline solution of NCNPs were correlated with the nitrogen doping content and nitrogen bonding state. The NCNPs also possessed excellent long-term durability and strong methanol tolerance in an alkaline solution compared to those of a commercial Pt/carbon catalyst." @default.
• W2511701116 created "2016-09-16" @default.
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• W2511701116 date "2015-01-01" @default.
• W2511701116 modified "2023-10-06" @default.
• W2511701116 title "From Cyano-aromatic Molecules to Nitrogen-doped Carbons by Solution Plasma for the Oxygen Reduction Reaction in Alkaline Medium" @default.
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• W2511701116 doi "https://doi.org/10.1016/j.matpr.2015.09.017" @default.
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