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• W2512505943 abstract "The catalytic activity of oxide-supported vanadium oxide is improved by the presence of tungsten oxide for the selective catalytic reduction of nitric oxides. We propose a mechanism for V–W synergy through studies of the reduction–oxidation behavior of near-monolayer VOX and WOX species grown by atomic layer deposition on the α-Al2O3 (0001) single crystal surface. In situ X-ray standing wave measurements reveal an overlayer of W6+ species that is correlated with the substrate lattice as well as a redox-reversible shift from uncorrelated V5+ to correlated V4+. X-ray photoelectron spectroscopy and electronic structure calculations show a partial reduction of W6+ in the presence of V4+, improving the Brønsted acidity in mixed V–W catalyst systems. This mechanism of V–W synergy suggests that control of W d-states might be used as a design parameter for Brønsted acid sites in multicomponent oxide catalysts." @default.
• W2512505943 created "2016-09-16" @default.
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• W2512505943 date "2015-07-02" @default.
• W2512505943 modified "2023-09-26" @default.
• W2512505943 title "Atomic-Scale View of VO_X–WO_X Coreduction on the α-Al₂O₃ (0001) Surface" @default.
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• W2512505943 doi "https://doi.org/10.1021/acs.jpcc.5b04802" @default.
• W2512505943 hasPublicationYear "2015" @default.
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