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- W2514896579 abstract "We present a microscopic semi-analytical theory for the description of organic molecules interacting strongly with a cavity mode. Exciton-vibration coupling within the molecule and exciton-cavity interaction are treated on an equal footing by employing a temperature-dependent variational approach. The interplay between strong exciton-vibration coupling and strong exciton-cavity coupling gives rise to a hybrid ground state which we refer to as the lower polaron-polariton. Explicit expressions for the ground state wavefunction, the zero-temperature quasiparticle weight of the lower polaron-polariton, the photoluminescence line strength, and the mean number of vibrational quanta are obtained in terms of the optimal variational parameters. The dependence of these quantities upon the exciton-cavity coupling strength reveals that strong cavity coupling leads to an enhanced vibrational dressing of the cavity mode, and meanwhile a vibrational decoupling of the dark excitons, which in turn results in a lower polaron-polariton resembling a single-mode dressed bare lower polariton in the strong coupling regime. Thermal effects on several observables are briefly discussed." @default.
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- W2514896579 date "2016-08-29" @default.
- W2514896579 modified "2023-10-17" @default.
- W2514896579 title "When polarons meet polaritons: exciton-vibration interactions in strongly-coupled organic microcavities" @default.
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