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• W2516053601 abstract "Abstract We present results from a joint theoretical and experimental study of the low‐energy Penning ionization of NH 3 , CH 3 F, and CHF 3 by metastable Ne( 3 P 2 ) and He( 3 S 1 ) atoms. We combine the merged neutral beams experiment, covering a range of collision energies between 0.1–150 K, with multichannel quantum defect theory calculations based on interaction potentials from symmetry‐adapted perturbation theory. The three symmetric tops provide several distinct properties that make them interesting targets for cold chemistry studies. Of these three, only NH 3 has a lone electron pair that leads to a strong binding with rare gas atoms. The CHF 3 molecule has much smaller rotational constants than both NH 3 and CH 3 F, and thus has a considerably higher density of rotational states already at low energies. Their presence opens inelastic collision channels that reduce the observed reactive cross section. We show that this effect dominates the total rate coefficient in heavy molecules already at relatively low collision energies but is much less prominent for lighter molecules" @default.
• W2516053601 created "2016-09-16" @default.
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• W2516053601 date "2016-09-09" @default.
• W2516053601 modified "2023-09-30" @default.
• W2516053601 title "Experimental and Theoretical Studies of Low‐Energy Penning Ionization of NH₃, CH₃F, and CHF₃" @default.
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• W2516053601 doi "https://doi.org/10.1002/cphc.201600608" @default.
• W2516053601 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27611761" @default.
• W2516053601 hasPublicationYear "2016" @default.
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