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- W2516478272 abstract "Global hetero- and homochiral polymorphous assemblies from an achiral fluorenone derivative were successfully constructed with multiple intermolecular hydrogen bonds by concentration modulation. Scanning tunneling microscopy investigations reveal that a heterochiral supramolecular double rosette-like structure was fabricated for the first time via hydrogen bond interactions with achiral 1-octanoic acid under low concentrations. When the solution concentration was increased, the structural transition from a heterochiral double rosette-like structure to a homochiral windmill-like pattern was observed. Interestingly, these two metastable structures ultimately could transform into a stable zigzag pattern at a bias voltage prompted by the STM tip. At high concentrations, only an achiral octamer arrangement could be obtained, owing to the changes of intermolecular hydrogen bonding, van der Waals force, and dipole–dipole interactions. The present results provided an important impetus for the induction and control of polymorphous chiral structural transformation through modulated solution concentration of achiral 1-octanoic acid." @default.
- W2516478272 created "2016-09-16" @default.
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- W2516478272 date "2015-07-29" @default.
- W2516478272 modified "2023-10-18" @default.
- W2516478272 title "Chiral Transition of the Supramolecular Assembly by Concentration Modulation at the Liquid/Solid Interface" @default.
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- W2516478272 doi "https://doi.org/10.1021/acs.jpcc.5b04799" @default.
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