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• W2517606987 abstract "Water-splitting dye-sensitized photoelectrochemical cells (WS-DSPECs) use a wide bandgap metal oxide semiconductor functionalized with a light-absorbing dye and water-oxidation catalyst to harvest light and drive water oxidation, respectively. We demonstrate here that the rutile polymorph of TiO2 (r-TiO2) is a promising anode material for WS-DSPECs. Recombination between the injected electron and oxidized sensitizer with r-TiO2 is an order of magnitude slower than with anatase TiO2 (a-TiO2), with injection yields approaching 100%. Studies with a reductive quencher demonstrate that r-TiO2 is significantly more efficient than a-TiO2, while exhibiting greater dye stability. Furthermore, comparison of direct band gap excitation photocurrent generation for bare and sensitized r-TiO2 suggests that the sensitizer functions as a light harvester and redox mediator." @default.
• W2517606987 created "2016-09-16" @default.
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• W2517606987 date "2016-08-25" @default.
• W2517606987 modified "2023-09-24" @default.
• W2517606987 title "Rutile TiO₂ as an Anode Material for Water-Splitting Dye-Sensitized Photoelectrochemical Cells" @default.
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• W2517606987 doi "https://doi.org/10.1021/acsenergylett.6b00279" @default.
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