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• W2520086836 endingPage "13183" @default.
• W2520086836 startingPage "13180" @default.
• W2520086836 abstract "A catalytic enantioselective route to C1- and C2-symmetric 2,2′-spirobiindanones has been realized through an intramolecular enolate C-acylation. This reaction employs a chiral ammonium counterion to direct the acylation of an in situ generated ketone enolate with a pentafluorophenyl ester. This reaction constitutes the first example of a direct catalytic enantioselective C-acylation of a ketone and provides an efficient and highly enantioselective route to axially chiral spirobiindanediones. These products can be diastereoselectively derivatized, offering access to a range of functionalized spirocyclic architectures." @default.
• W2520086836 created "2016-09-23" @default.
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• W2520086836 date "2016-10-06" @default.
• W2520086836 modified "2023-10-10" @default.
• W2520086836 title "Catalytic Enantioselective Synthesis of <i>C</i> ₁ - and <i>C</i> ₂ -Symmetric Spirobiindanones through Counterion-Directed Enolate <i>C</i> -Acylation" @default.
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• W2520086836 doi "https://doi.org/10.1002/anie.201607731" @default.
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