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- W2520235624 abstract "The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule level are long standing targets, however, they have been hampered by the limited spatial resolution in optical probing techniques. Here we investigate the electronic excitation of a single molecule with sub-molecular precision using a localised plasmon at the tip apex of a scanning tunnelling microscope (STM) as an excitation probe. Coherent energy transfer between the plasmon and molecular excitons is discovered when the plasmon is located in the proximity of isolated molecules, which is corroborated by a theoretical analysis. The polarised plasmonic field enables selective excitation of an electronic transition between anisotropic frontier molecular orbitals. Our findings have established the foundation of a novel single-molecule spectroscopy with STM, providing an integrated platform for real-space investigation of localised excited states." @default.
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- W2520235624 date "2017-07-05" @default.
- W2520235624 modified "2023-10-01" @default.
- W2520235624 title "Single-Molecule Investigation of Energy Dynamics in a Coupled Plasmon-Exciton System" @default.
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- W2520235624 doi "https://doi.org/10.1103/physrevlett.119.013901" @default.
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