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- W2520876949 abstract "A Gibbs free energy model for selective oxidation was developed which explains why Pt and Pd CO promoters produce NO x from HCN and NH 3 , the main products of coke burning. The model also predicts that base metal oxides are less likely to make NO x . High activity base metal CO promoters gave only marginally lower NO,, however. Experimental data then showed that high activity CO promoters are heat and mass transfer limited, leading to overheating of these microspheres with respect to the rest of the fluid bed. NO, selectivity was not improved for low activity Pt promoter, but lowering the activity of the base metal CO promoters gave ca. 50% lower NO x than Pt or Pd, in agreement with the Gibbs free energy model. A partial burn additive was also identified which has little CO oxidation activity, but converts HCN and NH 3 to N 2 at ca. 95% yield." @default.
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- W2520876949 date "2007-01-01" @default.
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- W2520876949 title "Toward a new generation of NOx additives" @default.
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