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• W2523161732 endingPage "6924" @default.
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• W2523161732 abstract "The complex Zintl phase Ca9Zn4.5Sb9 is a promising thermoelectric material due to its low thermal conductivity. Initial studies revealed that undoped Ca9Zn4.5Sb9 has a maximum zT value of 0.37 at 823 K. Hall effect measurements on Ca9Zn4.5–xAl2x/3Sb9 (x = 0, 0.5, 1), which nominally feature identical carrier concentration, suggested that control of the interstitial chemistry is critical in affecting the mobility of this system. Removal of the interstitial atoms results in rapid decrease in the carrier mobility, which has negative effects on the overall thermoelectric performance. Further material optimization was successfully carried out via Cu-doping in Ca9Zn4.5Sb9, with the aid of theoretical predictions. This resulted in high concentration of interstitial atoms as in Ca9Zn4.5–xCuxSb9 (x = 0.05, 0.1, 0.15, 0.2). For the optimized composition Ca9Zn4.35Cu0.15Sb9, a maximum of the figure of merit (zT = 0.72) was obtained at 873 K, which is increased by more than twice compared to the undoped material Ca9Zn4.5Sb9." @default.
• W2523161732 created "2016-09-30" @default.
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• W2523161732 date "2016-09-30" @default.
• W2523161732 modified "2023-10-15" @default.
• W2523161732 title "Tuning the Thermoelectric Properties of Ca₉Zn_4+<i>x</i>Sb₉ by Controlled Doping on the Interstitial Structure" @default.
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• W2523161732 doi "https://doi.org/10.1021/acs.chemmater.6b02498" @default.
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