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- W2526580448 abstract "A {open_quotes}one-pot{close_quotes} two-step catalytic synthesis of methanol in single fixed-bed continuous flow reactor from syngas via methylformate (MF) has been studied, and a CuZSM-5- or CuY-supported alkali-metal methoxides liquid/solid phases catalysts has been developed. Under conditions of 373K, 1.1MPa, H{sub 2}/CO/CH{sub 3}OH=8/5.8/1.7 (mol/mol), and GHSV=2250ml(STP)/h-g catal., X{sub CO} reached 37.5% and the net yield of CH{sub 3}OH reached 14.3mmol/h-g catal. The spectroscopic (ESR, XPS-Auger, TPR/TPO, and IR) characterizations of the catalyst systems provided significant experimental evidence for catalytically active species and reaction intermediates existing at the functioning catalysts. The mechanism of the catalysis and the major pathway of the reaction are discussed together with the results of the experimental investigation in the present work." @default.
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- W2526580448 date "1996-12-31" @default.
- W2526580448 modified "2023-09-23" @default.
- W2526580448 title "Study on catalytic synthesis of methanol from syngas via methylformate in heterogeneous {open_quotes}one-pot{close_quotes} reactions" @default.
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