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• W2527060944 abstract "Fluorescence optical rotary dispersion (F-ORD) is proposed as a novel chiral-specific and interface-specific spectroscopic method. F-ORD measurements of uniaxial assemblies are predicted to be fully electric-dipole-allowed, with corresponding increases in sensitivity to chirality relative to chiral-specific measurements in isotropic assemblies that are commonly interpreted through coupling between electric and magnetic dynamic dipoles. Observations of strong chiral sensitivity in prior single-molecule fluorescence measurements of chiral interfacial molecules are in excellent qualitative agreement with the predictions of the F-ORD mechanism and challenging to otherwise explain. F-ORD may provide methods to suppress background fluorescence in studies of biological interfaces, as the detected signal requires both polar local order and interfacial chirality. In addition, the molecular-level descriptions of the mechanisms underpinning F-ORD may also potentially apply to aid in interpreting chiral-specific Raman and surface-enhanced Raman spectroscopy measurements of uniaxially oriented assemblies, opening up opportunities for chiral-specific and interface-specific vibrational spectroscopy." @default.
• W2527060944 created "2016-10-07" @default.
• W2527060944 creator A5061854559 @default.
• W2527060944 creator A5080430957 @default.
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• W2527060944 date "2016-10-13" @default.
• W2527060944 modified "2023-10-14" @default.
• W2527060944 title "Theoretical Foundation for Electric-Dipole-Allowed Chiral-Specific Fluorescence Optical Rotary Dispersion (F-ORD) from Interfacial Assemblies" @default.
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• W2527060944 doi "https://doi.org/10.1021/acs.jpclett.6b01814" @default.
• W2527060944 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5310532" @default.
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• W2527060944 hasPublicationYear "2016" @default.
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