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- W2528069760 abstract "Abstract Borrowing hydrogen (or hydrogen autotransfer) reactions represent straightforward and sustainable C–N bond-forming processes. In general, precious metal-based catalysts are employed for this effective transformation. In recent years, the use of earth abundant and cheap non-noble metal catalysts for this process attracted considerable attention in the scientific community. Here we show that the selective N -alkylation of amines with alcohols can be catalysed by defined PNP manganese pincer complexes. A variety of substituted anilines are monoalkylated with different (hetero)aromatic and aliphatic alcohols even in the presence of other sensitive reducible functional groups. As a special highlight, we report the chemoselective monomethylation of primary amines using methanol under mild conditions." @default.
- W2528069760 created "2016-10-14" @default.
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- W2528069760 date "2016-10-06" @default.
- W2528069760 modified "2023-10-17" @default.
- W2528069760 title "Efficient and selective N-alkylation of amines with alcohols catalysed by manganese pincer complexes" @default.
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- W2528069760 doi "https://doi.org/10.1038/ncomms12641" @default.
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