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• W2528381085 abstract "Despite the enormous potential in bioinspired fabrication of high-strength structure by mimicking the spinning process of spider silk, currently accessible routes (e.g., microfluidic and electrospinning approaches) still have substantial function gaps in providing precision control over the nanofibrillar superstructure, crystalline morphology or molecular orientation. Here the concept of biomimetic nanofibrillation, by copying the spiders' spinning principles, was conceived to build silk-mimicking hierarchies in two-phase biodegradable blends, strategically involving the stepwise integration of elongational shear and high-pressure shear. Phase separation confined on nanoscale, together with deformation of discrete phases and pre-alignment of polymer chains, was triggered in the elongational shear, conferring the readiness for direct nanofibrillation in the latter shearing stage. The orderly aligned nanofibrils, featuring an ultralow diameter of around 100 nm and the rigid-soft system crosslinked by nanocrystal domains like silk protein dopes, were secreted by fine nanochannels. The incorporation of multiscale silk-mimicking structures afforded exceptional combination of strength, ductility and toughness for the nanofibrillar polymer composites. The proposed spider spinning-mimicking strategy, offering the biomimetic function integration unattainable with current approaches, may prompt materials scientists to pursue biopolymer mimics of silk with high performance yet light weight." @default.
• W2528381085 created "2016-10-14" @default.
• W2528381085 creator A5031207407 @default.
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• W2528381085 date "2016-10-03" @default.
• W2528381085 modified "2023-10-01" @default.
• W2528381085 title "Biomimetic Nanofibrillation in Two-Component Biopolymer Blends with Structural Analogs to Spider Silk" @default.
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• W2528381085 doi "https://doi.org/10.1038/srep34572" @default.
• W2528381085 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5046138" @default.
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• W2528381085 hasPublicationYear "2016" @default.
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