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- W2528899143 abstract "Abstract Designing uniformly dispersed Pd nanoparticles over nanoporous carbon supports is very demanding in the context of heterogeneous catalysis. However in most of the cases cluster/agglomerated Pd particles are formed over carbon matrixes, which lack sufficient stability and formation of a sustainable passive layer that can prevent the direct contact between the active metal sites with the reactants. Herein we report the in-situ preparation of surface-exposed Pd nanoparticle over N-doped carbon hollow tubes i.e. Pd@CHT, which showed high catalytic activity compared with agglomerated Pd on carbon. The simplicity in the preparation of Pd@CHT via one step direct carbonization of hypercrosslinked polymer tubes followed by reduction in the presence of NaBH 4 can offer huge potential in liquid phase heterogeneous catalysis. High dispersibility of the catalyst in the reaction medium, good stability and reusability of Pd@CHT is observed for the Sonogashira, cyanation and hydrogenation reactions for the synthesis of a wide range of value added fine chemicals, suggesting its future potential in heterogeneous catalysis." @default.
- W2528899143 created "2016-10-14" @default.
- W2528899143 creator A5031022550 @default.
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- W2528899143 date "2016-12-01" @default.
- W2528899143 modified "2023-10-16" @default.
- W2528899143 title "Surface-exposed Pd nanoparticles supported over nanoporous carbon hollow tubes as an efficient heterogeneous catalyst for the C C bond formation and hydrogenation reactions" @default.
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- W2528899143 doi "https://doi.org/10.1016/j.molcata.2016.09.037" @default.
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