FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2530968343> ?p ?o ?g. }

• W2530968343 endingPage "9808" @default.
• W2530968343 startingPage "9801" @default.
• W2530968343 abstract "We use liquid-phase transmission electron microscopy (LP-TEM) to characterize the structure and dynamics of a solution-phase superlattice assembled from gold nanoprisms at the single particle level. The lamellar structure of the superlattice, determined by a balance of interprism interactions, is maintained and resolved under low-dose imaging conditions typically reserved for biomolecular imaging. In this dose range, we capture dynamic structural changes in the superlattice in real time, where contraction and smaller steady-state lattice constants are observed at higher electron dose rates. Quantitative analysis of the contraction mechanism based on a combination of direct LP-TEM imaging, ensemble small-angle X-ray scattering, and theoretical modeling allows us to elucidate: (1) the superlattice contraction in LP-TEM results from the screening of electrostatic repulsion due to as much as a 6-fold increase in the effective ionic strength in the solution upon electron beam illumination; and (2) the lattice constant serves as a means to understand the mechanism of the in situ interaction modulation and precisely calibrate electron dose rates with the effective ionic strength of the system. These results demonstrate that low-dose LP-TEM is a powerful tool for obtaining structural and kinetic properties of nanoassemblies in liquid conditions that closely resemble real experiments. We anticipate that this technique will be especially advantageous for those structures with heterogeneity or disorder that cannot be easily probed by ensemble methods and will provide important insight that will aid in the rational design of sophisticated reconfigurable nanomaterials." @default.
• W2530968343 created "2016-10-21" @default.
• W2530968343 creator A5009669727 @default.
• W2530968343 creator A5045683824 @default.
• W2530968343 creator A5046262181 @default.
• W2530968343 creator A5064143115 @default.
• W2530968343 date "2016-10-17" @default.
• W2530968343 modified "2023-09-24" @default.
• W2530968343 title "<i>In Situ</i> Electron Microscopy Imaging and Quantitative Structural Modulation of Nanoparticle Superlattices" @default.
• W2530968343 cites W1804284596 @default.
• W2530968343 cites W1812643764 @default.
• W2530968343 cites W1863248722 @default.
• W2530968343 cites W1970360488 @default.
• W2530968343 cites W1977424326 @default.
• W2530968343 cites W1984147471 @default.
• W2530968343 cites W1986001908 @default.
• W2530968343 cites W1987521215 @default.
• W2530968343 cites W1989700141 @default.
• W2530968343 cites W1996520089 @default.
• W2530968343 cites W1998047469 @default.
• W2530968343 cites W2002052849 @default.
• W2530968343 cites W2004220723 @default.
• W2530968343 cites W2006563149 @default.
• W2530968343 cites W2007957644 @default.
• W2530968343 cites W2008521719 @default.
• W2530968343 cites W2028636490 @default.
• W2530968343 cites W2030280574 @default.
• W2530968343 cites W2035454388 @default.
• W2530968343 cites W2052109573 @default.
• W2530968343 cites W2060163612 @default.
• W2530968343 cites W2078833116 @default.
• W2530968343 cites W2084273768 @default.
• W2530968343 cites W2084588988 @default.
• W2530968343 cites W2087775507 @default.
• W2530968343 cites W2088133397 @default.
• W2530968343 cites W2089821515 @default.
• W2530968343 cites W2100473511 @default.
• W2530968343 cites W2105131183 @default.
• W2530968343 cites W2108711920 @default.
• W2530968343 cites W2109305701 @default.
• W2530968343 cites W2113012235 @default.
• W2530968343 cites W2113020843 @default.
• W2530968343 cites W2117441301 @default.
• W2530968343 cites W2127902738 @default.
• W2530968343 cites W2128383529 @default.
• W2530968343 cites W2131865769 @default.
• W2530968343 cites W2133934213 @default.
• W2530968343 cites W2136645442 @default.
• W2530968343 cites W2140690449 @default.
• W2530968343 cites W2142992372 @default.
• W2530968343 cites W2149705812 @default.
• W2530968343 cites W2156513210 @default.
• W2530968343 cites W2170425702 @default.
• W2530968343 cites W2173925994 @default.
• W2530968343 cites W2210611800 @default.
• W2530968343 cites W2214213576 @default.
• W2530968343 cites W2223101411 @default.
• W2530968343 cites W2262072985 @default.
• W2530968343 cites W2268896324 @default.
• W2530968343 cites W2312620520 @default.
• W2530968343 cites W2320412309 @default.
• W2530968343 cites W2321774739 @default.
• W2530968343 cites W2325382080 @default.
• W2530968343 cites W2325980328 @default.
• W2530968343 cites W2333002317 @default.
• W2530968343 cites W2338584008 @default.
• W2530968343 cites W2340247731 @default.
• W2530968343 cites W2416421032 @default.
• W2530968343 cites W2438516979 @default.
• W2530968343 cites W2560701883 @default.
• W2530968343 cites W3101549204 @default.
• W2530968343 cites W4232606260 @default.
• W2530968343 doi "https://doi.org/10.1021/acsnano.6b05270" @default.
• W2530968343 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27723304" @default.
• W2530968343 hasPublicationYear "2016" @default.
• W2530968343 type Work @default.
• W2530968343 sameAs 2530968343 @default.
• W2530968343 citedByCount "48" @default.
• W2530968343 countsByYear W25309683432017 @default.
• W2530968343 countsByYear W25309683432018 @default.
• W2530968343 countsByYear W25309683432019 @default.
• W2530968343 countsByYear W25309683432020 @default.
• W2530968343 countsByYear W25309683432021 @default.
• W2530968343 countsByYear W25309683432022 @default.
• W2530968343 countsByYear W25309683432023 @default.
• W2530968343 crossrefType "journal-article" @default.
• W2530968343 hasAuthorship W2530968343A5009669727 @default.
• W2530968343 hasAuthorship W2530968343A5045683824 @default.
• W2530968343 hasAuthorship W2530968343A5046262181 @default.
• W2530968343 hasAuthorship W2530968343A5064143115 @default.
• W2530968343 hasConcept C105382558 @default.
• W2530968343 hasConcept C120665830 @default.
• W2530968343 hasConcept C121332964 @default.
• W2530968343 hasConcept C132612359 @default.
• W2530968343 hasConcept C138631740 @default.
• W2530968343 hasConcept C146088050 @default.
• W2530968343 hasConcept C155672457 @default.
• W2530968343 hasConcept C159467904 @default.

• next