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• W2531337672 abstract "The transition-metal-free multicomponent coupling involving arynes, aromatic tertiary amines, and CO2 is reported. The reaction exhibits switchable selectivity depending on the electronic nature of the aromatic amines used. With amines bearing electron-releasing/neutral groups as the nucleophilic trigger, the reaction afforded 2-arylamino benzoates via a nitrogen to oxygen alkyl group migration. Employing electron-deficient amines in the reaction furnished 2-aminoaryl benzoates proceeding via the aryl to aryl amino group migration resembling a Smiles rearrangement." @default.
• W2531337672 created "2016-10-21" @default.
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• W2531337672 date "2016-10-13" @default.
• W2531337672 modified "2023-10-18" @default.
• W2531337672 title "Substrate-Controlled Selectivity Switch in the Three-Component Coupling Involving Arynes, Aromatic Tertiary Amines, and CO₂" @default.
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• W2531337672 doi "https://doi.org/10.1021/acs.orglett.6b02845" @default.
• W2531337672 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27736077" @default.
• W2531337672 hasPublicationYear "2016" @default.
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