FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2531985189> ?p ?o ?g. }

• W2531985189 endingPage "8120" @default.
• W2531985189 startingPage "8115" @default.
• W2531985189 abstract "The electrochemical reduction of CO2 into renewable chemical products such as formic acid is an important and challenging goal. Traditional Pd catalysts suffer from CO poisoning, which leads to current density decay and short operating lifetimes. Here we explored the ability to control Pd nanoparticle surface morphology to amplify catalytic activity and increase stability in the electroreduction of CO2 to formate. Through computational studies we have elucidated trends in intermediate binding which govern the selectivity and catalytic activity. We then rationally synthesized Pd nanoparticles having an abundance of high-index surfaces to maximize electrocatalytic performance. This catalyst displays a record current density of 22 mA/cm2 at a low overpotential of −0.2 V with a Faradaic efficiency of 97%, outperforming all previous Pd catalysts in formate electrosynthesis. The findings presented in this work provide rational design principles which highlight morphological control of high-index surfaces for the effective and stable catalytic electroreduction of CO2 to liquid fuels." @default.
• W2531985189 created "2016-10-28" @default.
• W2531985189 creator A5001195523 @default.
• W2531985189 creator A5012487063 @default.
• W2531985189 creator A5028992497 @default.
• W2531985189 creator A5051815230 @default.
• W2531985189 creator A5054680242 @default.
• W2531985189 creator A5060107939 @default.
• W2531985189 creator A5061135853 @default.
• W2531985189 date "2016-11-02" @default.
• W2531985189 modified "2023-10-09" @default.
• W2531985189 title "Rational Design of Efficient Palladium Catalysts for Electroreduction of Carbon Dioxide to Formate" @default.
• W2531985189 cites W1965362556 @default.
• W2531985189 cites W1971212285 @default.
• W2531985189 cites W1980921196 @default.
• W2531985189 cites W1981491642 @default.
• W2531985189 cites W1982891793 @default.
• W2531985189 cites W1992487468 @default.
• W2531985189 cites W2005872431 @default.
• W2531985189 cites W2007923221 @default.
• W2531985189 cites W2018942836 @default.
• W2531985189 cites W2032590691 @default.
• W2531985189 cites W2041511900 @default.
• W2531985189 cites W2049764985 @default.
• W2531985189 cites W2055252335 @default.
• W2531985189 cites W2078084378 @default.
• W2531985189 cites W2083222334 @default.
• W2531985189 cites W2087182232 @default.
• W2531985189 cites W2093202328 @default.
• W2531985189 cites W2093853901 @default.
• W2531985189 cites W2102743809 @default.
• W2531985189 cites W2112339932 @default.
• W2531985189 cites W2150687058 @default.
• W2531985189 cites W2167035995 @default.
• W2531985189 cites W2171162799 @default.
• W2531985189 cites W2254174122 @default.
• W2531985189 cites W2312983667 @default.
• W2531985189 cites W2318118246 @default.
• W2531985189 cites W2323309348 @default.
• W2531985189 cites W2326170978 @default.
• W2531985189 cites W2326928258 @default.
• W2531985189 cites W2336303331 @default.
• W2531985189 cites W4211160248 @default.
• W2531985189 doi "https://doi.org/10.1021/acscatal.6b01719" @default.
• W2531985189 hasPublicationYear "2016" @default.
• W2531985189 type Work @default.
• W2531985189 sameAs 2531985189 @default.
• W2531985189 citedByCount "260" @default.
• W2531985189 countsByYear W25319851892017 @default.
• W2531985189 countsByYear W25319851892018 @default.
• W2531985189 countsByYear W25319851892019 @default.
• W2531985189 countsByYear W25319851892020 @default.
• W2531985189 countsByYear W25319851892021 @default.
• W2531985189 countsByYear W25319851892022 @default.
• W2531985189 countsByYear W25319851892023 @default.
• W2531985189 crossrefType "journal-article" @default.
• W2531985189 hasAuthorship W2531985189A5001195523 @default.
• W2531985189 hasAuthorship W2531985189A5012487063 @default.
• W2531985189 hasAuthorship W2531985189A5028992497 @default.
• W2531985189 hasAuthorship W2531985189A5051815230 @default.
• W2531985189 hasAuthorship W2531985189A5054680242 @default.
• W2531985189 hasAuthorship W2531985189A5060107939 @default.
• W2531985189 hasAuthorship W2531985189A5061135853 @default.
• W2531985189 hasConcept C118792377 @default.
• W2531985189 hasConcept C127413603 @default.
• W2531985189 hasConcept C130349721 @default.
• W2531985189 hasConcept C147789679 @default.
• W2531985189 hasConcept C161790260 @default.
• W2531985189 hasConcept C171250308 @default.
• W2531985189 hasConcept C17525397 @default.
• W2531985189 hasConcept C178790620 @default.
• W2531985189 hasConcept C179104552 @default.
• W2531985189 hasConcept C185592680 @default.
• W2531985189 hasConcept C186460083 @default.
• W2531985189 hasConcept C192562407 @default.
• W2531985189 hasConcept C193115255 @default.
• W2531985189 hasConcept C24596552 @default.
• W2531985189 hasConcept C2777379063 @default.
• W2531985189 hasConcept C2780178953 @default.
• W2531985189 hasConcept C33989665 @default.
• W2531985189 hasConcept C42360764 @default.
• W2531985189 hasConcept C502130503 @default.
• W2531985189 hasConcept C512735826 @default.
• W2531985189 hasConcept C52859227 @default.
• W2531985189 hasConcept C53105671 @default.
• W2531985189 hasConceptScore W2531985189C118792377 @default.
• W2531985189 hasConceptScore W2531985189C127413603 @default.
• W2531985189 hasConceptScore W2531985189C130349721 @default.
• W2531985189 hasConceptScore W2531985189C147789679 @default.
• W2531985189 hasConceptScore W2531985189C161790260 @default.
• W2531985189 hasConceptScore W2531985189C171250308 @default.
• W2531985189 hasConceptScore W2531985189C17525397 @default.
• W2531985189 hasConceptScore W2531985189C178790620 @default.
• W2531985189 hasConceptScore W2531985189C179104552 @default.
• W2531985189 hasConceptScore W2531985189C185592680 @default.
• W2531985189 hasConceptScore W2531985189C186460083 @default.
• W2531985189 hasConceptScore W2531985189C192562407 @default.
• W2531985189 hasConceptScore W2531985189C193115255 @default.

• next